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- How to build a simple Luxeon LED bike headlight

Cree XLamp 7090 XR-E
The Cree XLamp 7090 XR-E is brighter than the Luxeon K2, and uses half the power. The only problem seems to be getting optics for them. Most of the available optics are intended for the 7090 XR which has a 100 degree beam, whereas the 7090 XR-E has a 75 degree beam. I've ordered some XR-Es and some lenses meant for the XR, and I'll see how well it works. I might end up having to wait another 3-6 months until the optics suppliers have new lenses available. I've probably used the same supplier as you, but I've had good service. They have been honest about delivery times and delays so far.
Regarding the difference in beam width between your commuting and mountain bike light, be aware that some optics are listed as full beam width, and some as half beam width. Some specify the beam width for monochromatic light. So the 6 degree Polymer Optics lens is actually 6 degree half angle, 12 degree full angle, and closer to 18 degree full angle with white light.